 | Sean Connery als James Bond |
 | Claudine Auger als Dominique 'Domino' Derval |
 | Adolfo Celi als Emilio Largo |
 | Luciana Paluzzi als Fiona Volpe |
 | Rik Van Nutter als Felix Leiter |
 | Guy Doleman als Count Lippe |
 | Molly Peters als Patricia Fearing |
 | Martine Beswick als Paula Caplan |
 | Bernard Lee als M |
 | Desmond Llewelyn als Q |
 | Lois Maxwell als Miss Moneypenny |
 | Roland Culver als Foreign Secretary |
 | Earl Cameron als Pinder |
 | Paul Stassino als Palazzi |
 | Rose Alba als Madame Boitier |
 | Philip Locke als Vargas |
 | George Pravda als Kutze |
| Michael Brennan als Janni |
 | Leonard Sachs als Group Captain |
 | Edward Underdown als Air Vice Marshall |
 | Reginald Beckwith als Kenniston |
| Harold Sanderson als Hydrofoil Captain |
 | Jack Gwillim als Senior RAF Staff Officer (uncredited) |
 | Suzy Kendall als Prue (uncredited) |
 | Mitsouko als Madame La Porte (uncredited) |
 | Philip Stone als SPECTRE Number 5 (uncredited) |
| Kevin McClory als Man Smoking at Nassau Casino (uncredited) |
 | Anthony Dawson als Ernst Stavro Blofeld (uncredited) |
 | Bob Simmons als Colonel Jacques Bouvar - SPECTRE #6 (uncredited) |
 | Richard Graydon als Largo's Henchman (uncredited) |
 | Michael Culver als Vulcan Bomber Crewman (uncredited) |
 | Barbara Jefford als Patricia Fearing (voice) (uncredited) |
 | André Maranne als SPECTRE #10 (uncredited) |
| Bob Simmons als Jacques Bouvar - SPECTRE #6 (uncredited) |
 | Nikki Van der Zyl als Dominique 'Domino' Derval (voice) (uncredited) |
| Terence Young | Director |
| Richard Maibaum | Screenplay |
| John Hopkins | Screenplay |
| Kevin McClory | Producer |
| John Barry | Original Music Composer |
| Ted Moore | Director of Photography |
| Ernest Hosler | Editor |
| Ken Adam | Production Design |
| Peter Murton | Art Direction |
| Anthony Mendleson | Costume Design |
| Kevin McClory | Story |
| Tom Jones | Theme Song Performance |
| Basil Newall | Makeup Artist |
| Paul Rabiger | Makeup Artist |
| Maurice Askew | Sound Recordist |
| Bert Ross | Sound Recordist |
| Jack Whittingham | Story |
| Jack Whittingham | Screenplay |
| Eileen Warwick | Hairdresser |
| David Middlemas | Production Supervisor |
| Gus Agosti | Assistant Director |
| Robert Watts | Second Assistant Director |
| Freda Pearson | Set Dresser |
| Michael White | Assistant Art Director |
| John Stears | Special Effects |
| Lamar Boren | Underwater Camera |
| Jimmy Spoard | Grip |
| John Winbolt | Camera Operator |
| John Brady | Wardrobe Master |
| Anthony Mendleson | Wardrobe Designer |
| Eileen Sullivan | Wardrobe Master |
| Peter R. Hunt | Supervising Editor |
| Frank Ernst | Location Manager |
| Willie Meyers | Location Scout |
| John Barry | Conductor |
| Derek Watkins | Musician |
| Joan Davis | Continuity |
| Albert R. Broccoli | Presenter |
| Maurice Binder | Main Title Designer |
| Lorraine Fennell | Publicist |
| Harry Saltzman | Presenter |
| Michael Reed | Second Unit Director of Photography |
| Dick Ziker | Stunts |
| Ian Fleming | Original Story |
| Peter R. Hunt | Editor |
