 | Sheridan Smith als Charmian Biggs |
 | Daniel Mays als Ronald Biggs |
 | Caroline Goodall als Muriel Powell |
 | Adrian Scarborough als Bernard Powell |
 | Tom Brooke als Mike Haynes |
 | Jack Lowden als Alan Wright |
 | Claire Rushbrook als Ruby Wright |
 | Leo Gregory als Eric Flower |
 | Ron Cook als Peter |
 | Iain McKee als Charlie Wilson |
 | Phil Cornwell als DS Jack Slipper |
 | Luke Newberry als Gordon |
 | Adrian Rawlins als DI Williams |
| Paul Whittington | Director |
| Jeff Pope | Writer |
| George Adams | Executive Producer |
| Kwadjo Dajan | Producer |
| Jeff Pope | Executive Producer |
| Tony Wright | Executive Producer |
| Bryony Marks | Original Music Composer |
| Fabian Wagner | Director of Photography |
| Mark Atkins | Editor |
| Ben Lester | Editor |
| Julie Harkin | Casting |
| Pat Campbell | Production Design |
| Ben Morieson | Art Direction |
| Nicole Northridge | Art Direction |
| Victoria McKenzie | Set Decoration |
| Elaine McLenachan | Set Decoration |
| Amy Roberts | Costume Design |
| Kitty Stuckey | Costume Design |
| Jenny Ward | Makeup Artist |
| Lesley Brennan | Makeup Artist |
