 | Richard Burton als Doctor Faustus |
 | Elizabeth Taylor als Helen of Troy |
 | Richard Durden als Evil Angel/Knight |
 | Michael Menaugh als Good Angel/Bishop |
| Andreas Teuber als Mephistopheles |
| Ram Chopra als Valdes |
| Richard Carwardine als Cornelius |
| Patrick Barwise als Wagner |
| David McIntosh als Lucifer |
| Jeremy Eccles als Belzebub |
 | Ian Marter als Pride/Emperor |
| Richard Burton | Director |
| Christopher Marlowe | Theatre Play |
| Gábor Pogány | Director of Photography |
| John DeCuir | Production Design |
| Peter J. Hall | Costume Design |
| John Shirley | Editor |
| Guy Luongo | Production Supervisor |
| Mario Nascimbene | Original Music Composer |
| Mario Nascimbene | Conductor |
| Nevill Coghill | Adaptation |
| Richard Burton | Producer |
| Richard McWhorter | Producer |
| Nevill Coghill | Director |
| Gus Agosti | Assistant Director |
| Roberto Cocco | Unit Manager |
| Boris Juraga | Art Direction |
| Elaine Schreyeck | Continuity |
| Carlo Lastricati | Production Assistant |
| Dario Simoni | Set Decoration |
| David Hildyard | Sound Mixer |
| John Aldred | Sound Mixer |
| Aldo De Martino | Sound |
| Augie Lohman | Special Effects |
| Brian West | Camera Operator |
| Ken Muggleston | Props |
| Les Wiggins | Sound Editor |
| Giannetto De Rossi | Makeup Artist |
| Agnes Flanagan | Hairdresser |
| Vasco Reggiani | Hairdresser |
| Ron Berkeley | Makeup Artist |
| Frank La Rue | Makeup Artist |
| Peter Harman | Special Effects |
